Is there a shortcut/key combination to change tool options?
e.g. when using the brush, pressing/holding a key and switching to weighted smoothing.
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There is indeed a way to do this, looking around shouldn't have taken long for you to figure this out either.
I don't think you can press and hold keys to do this (might be able to script it in somehow) but these work as toggle buttons to switch between each type of smoothing.